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Nea Smyrni is full of small parks and squares, usually at intersections where streets converge at odd angles. Because the area was outside of the city of Athens they had room to work with and made it as green and as open as was possible. It is for this reason that Nea Smyrni is considered one of the best urban areas in Athens.

Nea Smyrni is the home of the Panionios Football Club, the oldest in Greece, founded in 1890 in Smyrna, Ottoman Empire. They were also responsible for introducing basketball and volleyball to Greece. They play their games at Nea Smyrni Stadium which was built in 1940 which is also used for Track and Field and was the site of Metallica's first concert in Greece on June 27, 1993. The stadium is part of a huge complex of sports facilities, schools and the Church of the Metropolitan of Nea Smyrni
On the Square...
Chatzis is a pastry shop (ζαχαροπλαστείο) on the square of Nea Smyrni, close to Eleftheriou Venizelou street. Chatzis may be the best place to try oriental Greek sweets, like Baklava, Kataifi, and other deserts from Asia Minor. On the square, next to Chatzis, there is also a Starbucks, for those who prefer it.
Savvas apo to Monastiraki is next to Chatzis from the other side. You know the name because it is a souvlaki place with a long history. The first one opened in Monastiraki area in Athens sometime in the 1920s. Today it is a chain.
Lefteris and Giorgos are also places for souvlaki on the square. They have been in these locations for many years and the locals know and trust them. They can be considered almost traditional! To "go for souvlaki on the square" means to go to one of these two places!
Bar Aroma is a nice café/bar on the square with good coffee, drinks, sandwiches and other easy food and live music some nights. They normally play a selection of jazz, rock and blues.
Pizzoteca is a hip pizzeria on the square which also has some Italian dishes and deserts
Zuccherino is an elegant gelateria with great ice-cream and sweets that are difficult to resist!
Kenko Modish Sushi Bar at 22 El. Venizelou Ave at the top of the square and close to the Agia Fotinis Tram stop is a hip modern Japanese restaurant considered by many locals to be one of if not the best sushi restaurants in Athens. If it is closed try Koi Sushi Bar, a few blocks away at 71 Meg. Alexandrou, and like Kenko you should find the prices cheaper than those Japanese restaurants that are in the center of Athens.
Habit is an all-day café/bar on the square. Although it is open from the morning for coffee, its real face is revealed after 11 pm and even later, when it becomes Ellinadiko (like a disco that plays loud Greek contemporary music). Until 2-3 am or later it will be the only place around full of people. You can’t imagine what it is like if you go for a tranquil coffee in the morning with easy listening music, but late at night it will probably be packed with people, music playing full volume!!
Around Nea Smyrni...
Byzantio is a traditional kafenio on Eleftheriou Venizelou street across from the square. Go there for ouzo and meze or tsipouro if you prefer. Even a little house-wine with some meze will give you the essence of the Greek 50s!!
Bar Epitokio. Classic Rock Bar that has dedicated local customers as it has been open since 1987. It is located at the corner of Paleologou st and 60 Megalou Alexandrou st. One of the most popular hangouts in Nea Smyrni they play old style rock. There is a famous coffee shop called Nikos, open since 1976, just across frrom the Epitokio bar, and it is known for its meat pies and croissants.
Classic Nuveu is a Jazz Wine Bar with nice atmosphere, traditional jazz music and a rich wine list with gourmet snacks. You can find it on Eleftheriou Venizelou st across the square a little to your left (towards Neos Kosmos). The owner is Takis who also owns Epitokio.
The Café/Bar Aplika is a very nice chill out café with a cute garden and homemade sweets. It is open all day for breakfast or a snack anytime. It is located at the corner of Paleologou st and Megalou Alexandrou street across from Bar Epitokio.
On the corner of Venizelou and Omirou streets there is the Attika Bakery with the best bread you will ever eat as well as cakes and pastry and the usual stuff you will find in a Greek bakery. As in other neighborhoods there are bakeries all over and it is not out of the question that you will find one you like better. But this one is a good one to start with. It is part of the Attika Bakery chain but I believe this is the first one so this is where it all began.
If you are in the mood for Mexican food there is Amigos on the corner of Megalou Alexandrou st. and Korai st. Very nice place, some say authentic, with live Latin music some nights of the week.